Harindranath Chattopadhyaya was the son of Aghorenath Chattopadhyaya and younger brother of Sarojini Naidu and Virendranath Chattopadhyaya. Aghorenath had studied at Edinburgh University in the nineteenth century. Harindranath's parents were Bengalis who had settled in Hyderabad; Harindranath was born in the Deccan in 1898. Encouraged by his family, Harindranath began to write verse as a child and also enjoyed acting.
He married Kamaladevi, a Madrasi widow in 1919, having been introduced by a younger sister, Suhasini. Shortly after their marriage, Harindranath sailed to England, leaving behind his wife (who was later to join him). Harindranath had published poems and written plays in India before he arrived in London, and was helped to settle in Britain by friends of his famous elder sister, Sarojini. He initially lodged in Gower Street and sent his poems to Cambridge in order to gain admission as a research scholar. Harindranath successfully gained admission into Fitzwilliam Hall and took up research work on 'William Blake and the Sufis'. During his time as a student in Britain, Harindranath's poems were published in the Indian Magazine (Journal of the National Indian Association) and Britain and India (Journal of the Theosophical-influenced Britain and India Association). He corresponded with Laurence Binyon about publishing further anthologies of poems in London.
As the Civil Disobedience movement gained momentum in India, Harindranath and Kamaladevi decided to return to India and Harindranath abandoned his Cambridge degree. They returned via Europe to visit with his elder brother, the revolutionary Virendranath Chattopadhyaya (Chatto) and also met with Madame Cama.
In 1929, a publication entitled Five Plays was produced by Fowler Wright in London. The book printed praise inside its front cover from Rabindranath Tagore, Alice Meynell and George Russell (AE) (for Harindranath's poetry). The playlets (adapted from Hindu mythology) were introduced by S. Fowler Wright, who compared Harindranath Chattopadhyaya to Joseph Conrad. Harindranath's play, 'Tukaram' had been performed in the Little Theatre, London, in 1928. Harindranath maintained a successful career as poet, playwright and actor upon his return to India. He died in 1990.